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4 3.2.8 Isotherms ................................................................................................. 15 Modelling and Simulation......................................................................... 17 5 4.4.2 Multisite Langmuir parameters estimation ......................................................... 44 Conclusions ......................................................................................... 47 5.1 Accomplished goals .......................................................................... 47 5.2 Limitations and future work ............................................................... 48 4.1 4.1.1 4.1.2 4.2 4.2.1 4.2.2 4.2.3 4.3 4.3.1 4.3.2 4.4 Breakthrough model validation ........................................................... 17 Axial dispersion model ................................................................................. 18 Multilayer model ........................................................................................ 19 Langmuir-Freundlich multilayer isotherm .............................................. 21 Langmuir-Freundlich isotherm modeling............................................................ 22 Langmuir-Freundlich multilayer isotherm validation ............................................. 23 Validation of the Langmuir-Freundlich multilayer isotherm with different data ............ 31 Multisite Langmuir isotherm ............................................................... 33 Multisite Langmuir isotherm modeling .............................................................. 34 Multisite Langmuir simulations ....................................................................... 35 Parameter estimation ....................................................................... 38 Parameter estimation of the LDF coefficients for the process using Langmuir-Freundlich 4.4.1 isotherm ............................................................................................................ 39 Appendix 1 Pressure Swing Adsorption Milestones ............................................. 52 Appendix 2 gPROMS® Adsorption Models......................................................... 53 2.1 List of models and specifications ......................................................... 53 Appendix 3 Langmuir-Freundlich Isotherm ...................................................... 55 3.1 Langmuir-Freundlich isotherm modelling ............................................... 55 3.2 Adsorbents and bed properties............................................................ 57 3.3 Five component mixtures breakthrough simulations ................................. 59 3.4 Validation of the Langmuir-Freundlich multilayer isotherm with different data 61 Appendix 4 Multisite Langmuir Isotherm ......................................................... 63 4.1 Multisite Langmuir isotherm modelling .................................................. 63 Pressure Swing Adsorption for Hydrogen Purification iiPDF Image | PRESSURE SWING ADSORPTION FOR THE PURIFICATION OF HYDROGEN
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