TEMPERATURE SWING ADSORPTION PROCESSES FOR GAS SEPARATION

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TEMPERATURE SWING ADSORPTION PROCESSES FOR GAS SEPARATION ( temperature-swing-adsorption-processes-for-gas-separation )

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2.2.8 Product purity and yield......................................................................40 2.3 Optimization of geometry and material selection ........................................41 2.3.1 Adsorbent microchannel geometry......................................................41 2.3.2 Adsorbent and HTF material selection ................................................49 2.4 2.5 3 3.1 Results .......................................................................................................56 Conclusions................................................................................................65 PERFORMANCE ASSESSMENT .........................................................68 Introduction................................................................................................68 3.3 3.4 3.5 3.6 3.7 3.8 3.9 4 4.1 4.2 4.3 Process performance prediction ..................................................................74 Energy requirements and operating cost .....................................................79 Reduction in operating energy requirement ................................................82 Heat recovery from the cooling stage..........................................................86 Discussion..................................................................................................89 Multistage purification process...................................................................94 Summary and Conclusions .........................................................................96 EXPERIMENTS AND MODEL VALIDATION....................................98 Introduction................................................................................................98 Experimental set-up and procedure...........................................................102 Experimental results and discussion .........................................................107 System design selection and results ............................................................69 3.2 3.2.1 Liquid HTF recirculation and absorption ............................................69 4.4 4.4.1 Adsorbent-coated microchannel equations ........................................116 4.4.2 Header equations ..............................................................................126 4.4.3 Valve equations ................................................................................128 4.4.4 Source and sink models ....................................................................128 4.4.5 Simulation procedure........................................................................128 4.5 Model validation ......................................................................................129 Model development ..................................................................................115 vii

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