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(a) (b) Figure 4.6: Efficiencies of CO2 dissociation over all flow rates: a) energy efficiency, and b) conversion efficiency. dominant mechanism of dissociation in this system. The one-step collisional process described in Equation 3.43 requires the electron energy to exceed 8 eV for dissociation to occur, which greatly exceeds the OC=O bond energy. This dissociation mechanism is typically dominant in low-pressure discharges with high values of reduced electric field, which describes the operating conditions used in this experiment. The high electron energies required give rise to the excitation of various other states that do not contribute to dissociation, resulting in low energy efficiency. Also, it is unlikely that helicon mode was ever reached during operation; most likely the discharge remained in capacitive or inductive mode. The operating pressure range on the order of 100 mtorr was too high to excite the helicon mode structure, which typically appears around 1 mtorr with power levels greater than 1 kW based on previous experiments using the experimental setup [60]. This experiment was limited to only 1 kW of input power. Thus, the high electron density characteristic of a helicon plasma was not present to help increase the electron impact events resulting in dissociation. 75PDF Image | CO2 Conversion in a Microwave Plasma Catalyst System
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