CO2 Conversion in a Microwave Plasma Catalyst System

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CO2 Conversion in a Microwave Plasma Catalyst System ( co2-conversion-a-microwave-plasma-catalyst-system )

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CHAPTER VI Results and Discussion The results of experimental and computational work performed for the systems described in Chapter V will now be presented. First in Section 6.1 the results of CO2 dissociation in the plasma system alone will be discussed along with the plasma properties derived from OES measurements. Next the results of the plasma/catalyst system along with the control test using an uncoated monolith inserted into the plasma will be shown in Section 6.2. A comparison of computational results from GlobalKin simulations with the pure plasma system is given in Section 6.3. A discussion of all results will follow in Section 6.4 along with a cost analysis comparison of existing technological approaches. Lastly a summary of the experimental and computational work will be given in Section 6.5. 6.1 Plasma System Results 6.1.1 Initial Plasma Observations The experimental parameters that were varied include microwave input power, CO2 flow rate, and Ar flow rate. In order to sustain a discharge with CO2 flow rates greater than 1 slm, microwave power is required to be equal to or exceed 1 kW. Thus, the power level ranged from 1-2 kW for all tests. As described in Section 5.1, the ideal value for specific energy input to achieve energy efficient dissociation is around 107

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