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Chapter 2 Hydrogen radical assisted conversion of Carbon dioxide to methane Abstract In this work the efficiency of conversion of carbon dioxide to methane (methanation) using H radicals is reported. Also in non-equilibrium environments, for efficient conversion of CO2 to methane, a syngas (CO + H2) like intermediate is shown to be a prerequisite; the underlying mechanisms were inferred by measuring the product distributions quantitatively using infrared laser absorption spectroscopy and quadrupole mass spectrometry, and comparing them with product distributions obtained with CO as carbon precursor. Oxygen radical, also produced in the process, reduces the efficiency of CO2 methanation by binding H and forming water. Both observations point to necessity of spatial separation of the CO2 dissociation step and the association of H with carbon for efficient methanation. The importance of surface reactions and the requirement for new catalysts suited for radical assisted conversion of CO2 to methane is demonstrated with copper and aluminium as examples. 17PDF Image | Understanding CO2 containing non-equilibrium plasmas
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