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4.3. REACTION KINETICS MODEL 4. FLUID MODELLING OF CO2 DISSOCIATION E30, E31 E32, E33 E34, E35 E36, E37 CO2(v2b) + e ←−→ CO2(v4)+ e CO2(v2b) + e ←−→ CO2(v5) + e CO2(v31)+ e ←−→ CO2(v32)+ e CO2(v4)+ e ←−→ CO2(v5) + e f(Ue) f(Ue) f(Ue) f(Ue) Analogous to E2 [176] Analogous to E4+E6 [176] Analogous to E8 [176] Analogous to E2 [176] [176] [176] [175] [175] [175] [175] [181] [181]† [181]† [181]† [181]† [181]† [181]† [109] [168] [182] [183] [167] Electron impact excitation and de-excitation of electronically excited states E38, E39 CO2(v0) + e ←−→ CO*2 + e E40,E41 CO (v0)+e ←−→ CO** +e Electron impact dissociation E42 CO2(v0)+e −−→ CO+O+e Electron impact ionization and detachment E43 CO2(v0)+e −−→ CO+2 +e+e E44 CO2(v0)+e −−→ CO+2(A)+e+e E45 CO2(v0) + e −−→ CO+2(B)+ e + e E46 O– + e −−→ O + e + e Dissociative electron attachment E47 CO2(v0)+e−−→CO+O– E48 CO2(v1) + e −−→ CO +O– E49 CO2(v2a)+e−−→CO+O– E50 CO2(v2b)+e−−→CO+O– E51 CO2(v31)+ e −−→ CO + O– E52 CO2(v4)+ e −−→ CO + O– E53 CO2(v5)+e−−→CO+O– Dissociative electron-ion recombination E54 CO+2 + e −−→ CO + O Collisional and associative detachment E56 O– + CO2(v0) −−→ O + CO2(v0) + e E57 O– + CO −−→ CO2(v2b)+ e E58 O– + O −−→ O2 + e E59 O–2 + O −−→ O3 + e f(Ue) f(Ue) f(Ue) f(Ue) f(Ue) f(Ue) [179, 180] f(Ue), Kat(Ue) f(Ue), Kat(Ue) f(Ue), Kat(Ue) f(Ue), Kat(Ue) f(Ue), Kat(Ue) f(Ue), Kat(Ue) f(Ue), Kat(Ue) 4.2 × 10−13 (Te /300)−0.75 4.0 × 10−18 5.8 × 10−15(Tg)−0.4 2.3 × 10−16 1.5 × 10−16 22 In addition to the collision processes involving electrons, further 239 heavy particle collision processes and four radiation processes are considered. In order to allow for an analysis of the vibrational energy transfer, an extended set of reactions describing the vibrational-translational (VT) and vibrational-vibrational (VV) relaxation processes is used. The corresponding reactions and rate coefficients are listed in tables 4.3 and 4.4. Furthermore, 16 collisions between neutrals in their ground state, non-detaching ion- neutral reactions such as charge transfer reactions as well as ion-ion recombination pro- cesses are taken into account as given in table 4.5. In this table the two radiation processes (from excited ions) are listed as well. 85PDF Image | Understanding CO2 containing non-equilibrium plasmas
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