Understanding CO2 containing non-equilibrium plasmas

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Understanding CO2 containing non-equilibrium plasmas ( understanding-co2-containing-non-equilibrium-plasmas )

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4. FLUID MODELLING OF CO2 DISSOCIATION 4.3. REACTION KINETICS MODEL Table 4.3: Vibrational-translational relaxation reactions considered in the model. The rate coefficients refer to a gas temperature of 400 K and are given in m3s−1.†:j=3,...,20;cj =j−2. Number Reaction VT1 CO2(v1) + CO2(v0) −−→ CO2(v0) + CO2(v0) VT2 CO2(v2b) + CO2(v0) −−→ CO2(v1) + CO2(v0) VT3 CO2(v2a) + CO2(v0) −−→ CO2(v0) + CO2(v0) VT4 CO2(v2a) + CO2(v0) −−→ CO2(v2b) + CO2(v0) VT5 CO2(v31) + CO2(v0) −−→ CO2(v0) + CO2(v0) VT6 CO2(v31) + CO2(v0) −−→ CO2(v1) + CO2(v0) VT7 CO2(v31) + CO2(v0) −−→ CO2(v4) + CO2(v0) VT8 CO2(v32) + CO2(v0) −−→ CO2(v31) + CO2(v0) VT9 CO2(v4)+ CO2(v0) −−→ CO2(v2b) + CO2(v0) VT10 CO2(v4)+ CO2(v0) −−→ CO2(v1) + CO2(v0) VT11 CO2(v5) + CO2(v0) −−→ CO2(v4)+ CO2(v0) VT12 CO2(v5) + CO2(v0) −−→ CO2(v31) + CO2(v0) VT13 CO2(v5) + CO2(v0) −−→ CO2(v2b) + CO2(v0) VT14 CO2(v6) + CO2(v0) −−→ CO2(v5) + CO2(v0) VT15 CO2(v6) + CO2(v0) −−→ CO2(v4)+ CO2(v0) VT16 CO2(v7) + CO2(v0) −−→ CO2(v6) + CO2(v0) VT17 CO2(v8) + CO2(v0) −−→ CO2(v7) + CO2(v0) VT18–VT35 CO2(v3j) + CO2(v0) −−→ CO2(v3(j−1)) + CO2(v0) Rate coefficient 1.06 × 10−20 2.15 × 10−20 9.68 × 10−20 6.92 × 10−17 1.0 × 10−23 1.66 × 10−23 6.04 × 10−21 5.0 × 10−23 3.20 × 10−20 8.96 × 10−24 6.46 × 10−20 1.72 × 10−22 5.95 × 10−26 9.62 × 10−20 2.65 × 10−23 2.12 × 10−20 3.18 × 10−20 cj × 10−22 Reference [184] [184] [184, 185] [185] [36] [184] [184] [36] [184] [184] [184] [184] [184] [184] [184] [184] [184] [36]† Table 4.4: Table of vibrational energy exchange reactions used in the model. The rate coefficients refer to a gas temperature of 400 K and are given in m3 s−1 . †:i=2,...,19;‡j=2,...,i;ci =10fori≤9;ci =(19−i)for10≤i≤ 15;ci =(20−i)for16≤i≤19. Number Reaction VV1 CO2(v2b) + CO2(v0) −−→ CO2(v1) + CO2(v1) VV2 CO2(v31) + CO2(v31) −−→ CO2(v32) + CO2(v0) VV3 CO2(v32) + CO2(v31) −−→ CO2(v33) + CO2(v0) VV4 CO2(v4) + CO2(v1) −−→ CO2(v2b) + CO2(v2b) VV5 CO2(v4) + CO2(v4) −−→ CO2(v2b) + CO2(v5) VV6 CO2(v5) + CO2(v0) −−→ CO2(v4) + CO2(v1) VV7 CO2(v5) + CO2(v1) −−→ CO2(v4)+ CO2(v2b) VV8 CO2(v5) + CO2(v2b) −−→ CO2(v4)+ CO2(v4) VV9 CO2(v6)+ CO2(v0) −−→ CO2(v5) +CO2(v1) VV10 CO2(v6)+ CO2(v1) −−→ CO2(v5) + CO2(v2b) VV11 CO2(v6) + CO2(v2b) −−→ CO2(v5) + CO2(v4) VV12 CO2(v7) + CO2(v0) −−→ CO2(v6) +CO2(v1) Rate coefficient 1.01 × 10−18 1.0 × 10−16 1.0 × 10−16 2.99 × 10−18 8.30 × 10−17 3.07 × 10−18 6.03 × 10−18 9.24 × 10−18 4.58 × 10−18 9.24 × 10−18 1.52 × 10−17 2.76 × 10−16 Reference [184] [36] [36] [184] [185] [184] [184] [184] [184] [184] [184] [185] 86

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