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4.3. REACTION KINETICS MODEL 4. FLUID MODELLING OF CO2 DISSOCIATION VV13 VV14 VV15 VV16-VV33 VV34-VV204 CO2(v7) + CO2(v1) −−→ CO2(v6) + CO2(v2b) CO2(v8) + CO2(v0) −−→ CO2(v7) +CO2(v1) CO2(v5) + CO2(v5) −−→ CO2(v4)+ CO2(v6) CO2(v3i) + CO2(v31) −−→ CO2(v3(i+1)) + CO2(v0) CO2 (v3i ) + CO2 (v3j ) −−→ CO2 (v3(i+1) ) + CO2 (v3(j−1) ) 5.53 × 10−16 1.31 × 10−15 1.30 × 10−15 1 × 10−16 ci × 10−17 [185] [185] [185] [36]† [36]†‡ 4.5: Neutral-neutral, ion-neutral and ion-ion collision processes as well as radiative transition processes used in the model. The rate-coefficients have the units of m3s−1 for two-body collisions, m6s−1 for three-body collisions and s−1 for radiative transitions. The gas temperature Tg is given in K. Table Number Reaction Neutral kinetics of ground state particles N1 CO2(v0)+O −−→ CO+O2 N2 CO+O2 −−→ CO2(v0)+O N3 CO + O + CO2(v0) −−→ CO2(v0) + CO2(v0) N4 O2+O3 −−→O2+O2+O Rate coefficient 2.8 × 10−17 exp(−26500/Tg) 4.2 × 10−18 exp(−24000/Tg) 1.6 × 10−45 exp(−1510/Tg) 7.26 × 10−16 exp(−11400/Tg) 1.7×10−42T−1.2 Reference [107] [107] [161] [183] [161] [186] [183] [186] [63] [163] [167] [167] [167] [167] [163] [163] [187] [187] N5 O +O+CO (v0) −−→ O +CO (v0) 2232g N6 O +O+O −−→ O +O 8.61×10−43T−1.25 2232 g N7 O2 +O+O −−→ O3 +O N8 O3 + O −−→ O2 + O2 N9 O + O + CO (v0) −−→ O + CO (v0) 222g Ion-atom and ion-molecule reactions (including charge transfer) I1 O– + CO2(v0) + CO2(v0) −−→ CO–3 + CO2(v0) I2 O–2 + CO2(v0) + CO2(v0) −−→ CO–4 + CO2(v0) I3 O –2 + O −−→ O 2 + O – I4 CO–3 +O −−→ O–2 +CO2(v0) I5 CO–4 + O −−→ CO–3 + O2 Ion-ion recombination I6 CO+2 + CO–3 −−→ CO2(v0) + CO2(v0) + O I7 CO+2 + CO–4 −−→ CO2(v0) + CO2(v0) + O2 Radiative transitions R1 CO+2(A) −−→ CO+2 +hν R2 CO+2(B) −−→ CO+2 +hν 9.0 × 10−41 1.2 × 10−40 1.5 × 10−16 1.1 × 10−16 1.4 × 10−16 5.0 × 10−13 5.0 × 10−13 6.1 × 106 7.2 × 106 2.15×10−40 exp(345/Tg) 1.81 × 10−17 exp(−2300/Tg ) 3.81 × 10−42T−1.0 exp(−170/Tg) 87PDF Image | Understanding CO2 containing non-equilibrium plasmas
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