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4.6. CONCLUSION 4. FLUID MODELLING OF CO2 DISSOCIATION Conversion frequency – the ratio of amount of CO produced per unit time to the CO2 present in the reactor – is used to compare between the experiments, which involve a flow and the one-dimensional model which does not. Just as in the experiment, conver- sion frequency increases monotonically with specific energy input, regardless of the set of operational parameters used. While the specific energy input matched very well with the experiment, a deviation was clearly noticed with respect to CO2 conversion; CO2 con- version is the conversion frequency scaled to the corresponding residence times reported in the experiments. The discrepancy in the conversion can be easily explained when the dissociation from electronically excited molecules is considered. The results presented in the work can be used to explore the important electronic states which hitherto neglected, but might prove to be important in CO2 dissociation. Acknowledgment The work was partly supported by the German research foundation within the Collabor- ative Research Centre Transregio 24 and under grant LO 623/3-1. The numerical code (fluid model) used in this chapter was developed by Dr. M.M. Becker in the group of Priv. -Doz. Dr. D. Loffhagen from INP Greifswald. The electron kinetic data was sup- plied by Priv. -Doz. Dr. D. Loffhagen. Most of the work was done under the guidance and support from Dr. Becker and Dr. Loffhagen including during one month stay in their group. The computational resources were made available from Applied Physics Depart- ment at TU Eindhoven; support of Dr. A. Bol and Prof. W. M. M. Kessels in this regard is greatly appreciated. 105PDF Image | Understanding CO2 containing non-equilibrium plasmas
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